A comprehensive understanding of ground and optically-excited hyperfine structure of ¹⁶⁷Er³+:Y2SiO5

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dc.contributor.authorHorvath SP
dc.contributor.authorRakonjac JV
dc.contributor.authorChen Y-H
dc.contributor.authorLongdell JJ
dc.contributor.authorGoldner P
dc.contributor.authorWells J-PR
dc.contributor.authorReid MF
dc.date.accessioned2018-10-08T23:23:34Z
dc.date.available2018-10-08T23:23:34Z
dc.date.issued2018en
dc.date.updated2018-09-14T10:36:42Z
dc.description.abstractUsing high-performance computing techniques and targeted experimental investigation we have developed a predictive crystal-field model of the complex hyperfine structure of ¹⁶⁷Er³+:Y2SiO5 We simultaneously match site-selective spectroscopic data up to 20,000 cm-¹, rotational Zeeman data, and ground- and excited-state hyperfine structure determined from high-resolution Raman-heterodyne spectroscopy on the 1.5 μm telecom transition. We achieve agreement of better than 50 MHz for assigned hyperfine transitions. The successful analysis of the complex hyperfine patterns opens the possibility of systematically searching this whole class of materials for the ZEFOZ transitions that have proved so useful in quantum information applications.en
dc.identifier.urihttp://hdl.handle.net/10092/16100
dc.language.isoen
dc.subjectquant-phen
dc.subjectquant-phen
dc.subject.anzsrcField of Research::03 - Chemical Sciences::0306 - Physical Chemistry (incl. Structural)::030606 - Structural Chemistry and Spectroscopyen
dc.subject.anzsrcField of Research::03 - Chemical Sciences::0307 - Theoretical and Computational Chemistry::030701 - Quantum Chemistryen
dc.subject.anzsrcField of Research::03 - Chemical Sciences::0302 - Inorganic Chemistry::030207 - Transition Metal Chemistryen
dc.titleA comprehensive understanding of ground and optically-excited hyperfine structure of ¹⁶⁷Er³+:Y2SiO5en
dc.typeJournal Articleen
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